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Blog Radioactivity fun!
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Engagement
  • Author Author: neuromodulator
  • Date Created: 15 Sep 2020 4:32 AM Date Created
  • Views 278 views
  • Likes 11 likes
  • Comments 8 comments
  • provingsciencech
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Radioactivity fun!

neuromodulator
neuromodulator
15 Sep 2020

  • Introduction
  • The Geiger counter setup
  • Background radiation
  • Radiation distance
  • Radiation blocking
  • Final words

Introduction

 

Radioactive decay is the process where unstable atoms lose energy through emission of ionizing radiation in the form of particles or photons (gamma radiation). When unstable atoms emit particles they their nucleus changes, which means that the atom transmutes into a different isotope or different element. Ionizing radiation has enough energy to detach electrons from atoms and in that way generate ions. Chemical bonds and reactions depend solely on electrons and for that reason, ionizing radiation can affect chemical bonds, which can degrade materials, but also, in the case of organisms, cause cell or DNA damage (or in the worse case: cancer). Ionizing radiation can be found everywhere, from cosmic rays, to UV light, to radiation generated by naturally occurring radioactive elements. Luckily for us, we have multiple mechanism that make it relatively hard to develop cancer, even if our DNA gets damaged by ionizing radiation.

 

There are multiple techniques to measure radiation, with capabilities to measure different properties of the radiation, such as its direction, its energy and its type. One of these techniques is the Geiger counter, which only "counts" ionizing radiation events. The main component of the Geiger counter is the Geiger tube, which is a tube filled with a gas mixture to which high voltage (~400 V) is applied. The tube is non-conductive, but once a radioactivity event occurs within the chamber, the gas mixture turns conductive for a very short period (~1 ms). "Classic" Geiger counters emitted a "tick" sound once these event occurred, which depending on the rate, indicated the amount of radiation detected by the tube.

 

In this project I used a Geiger counter to measure background radiation, to perform some mathematical analyses and also see how different conditions (such as the distance from the tube of a radioactive fossil) affect the count rate.

 

 

The Geiger counter setup

 

For the Geiger counter I used a SBM-20 (СБМ-20) tube, which I bought for less than 10 USD on ebay long ago. These tubes were produced in the Soviet Union during cold war, they have a length of 108 mm, a diameter of 11 mm, use a gas mixture of Neon, Bromine and Argon and require a voltage between 350 and 475 V, and when they detect an event they turn conductive for ~0.5 ms.

 

 

 

The setup that I build to make the measurements looked like this:

 

 

 

Voltage is boosted from 6 V to  400 V, and supplied to the Geiger tube. When a ionizing radiation event occurs, current flows through a Mega-ohm range voltage divider and feed to  an MCU ADC through a buffer. The MCU samples at ~18 kHz and sends through a virtual serial port the time when the event occurred to the SBC, which stores the data into a file.

 

To avoid affecting the measurements I taped the tube to the bench:

 

 

 

Background radiation

 

Radioactivity is everywhere, so the first thing that I did was to measure the radioactivity at my bench. I measured 68,043 counts during a 38.2 h period, which gave me rate of 29.7 CPM (Counters Per Minute), I also measured the 95% confidence interval of the rate, which was from 29.5 to 29.9 CPM.

 

Lets talk a bit about the statistical aspects of the radioactivity events. Radioactive decay events are random and are not affected by external conditions (Temperature, pressure, magnetic or electric fields, etc.). Unless the materials that are radioactively decaying have short decay constant or half-life, the radiation events should occur at relatively constant rate (when measuring it using a large number of events in a long time window). These events can be modeled as a Poisson point process, which is a stochastic process that can be specified with a single parameter: the rate of the points, which species the average density of the points.

 

The distribution of the intervals of a Poisson point process have an exponential distribution, which can be specified with a single rate parameter as well. Since the tube can't detect 2 events with a time separation of < 0.5 ms, the Poisson point process (and the interval exponential distribution) can't perfectly describe the captured data, but at low levels of radiation the chance that 2 events occur with a separation of < 0.5 ms is still quite low.

 

At this point it was time to test the theory, so I generated an histogram of the interval times and normalized it to generate an empirical probability distribution function (PDF), which was compared to the exponential PDF at 29.7 CPM.

 

 

Then I did the same, but with the cumulative distribution function (CDF).

 

 

 

The empirical data matched really well the theory, but to perform more objective tests there are goodness of fit methods such as the Kolmogorov-Smirnov test, but I didn't want to make this blog post more boring. One last thing that I wanted to quickly and roughly check, was if the counting rate changed during time (or technically if the process was stationary), So i plotted the CPM rate for every hour:

 

 

And as it can be seen, at least in this time window, the process appears to be stationary.

 

 

Radiation distance

 

Of all common objects that I have in the house I found just one that produce a very noticeable count rate increase: a fossilized bone. It generated 237.5 CPM, with a 95% confidence interval of 236.5 - 238.7 CPM when layed over the tube in direct contact with it.

 

 

 

The rest of the object that I tried could barely increase twice the counting rate.

 

Next I wanted to see how the distance affected the measured radiation. So I measured the rate by separating the fossil from the tube at a distances of 2, 4, 8, 16 and 32 cm:

 

Absolute CPM

Background: Mean: 29.7 CPM, CI95: 29.5 - 29.9

02 cm:      Mean: 81.0 CPM, CI95: 80.4 - 81.5

04 cm:      Mean: 57.2 CPM, CI95: 56.7 - 57.6

08 cm:      Mean: 40.8 CPM, CI95: 40.5 - 41.2

16 cm:      Mean: 33.3 CPM, CI95: 33.0 - 33.6

32 cm:      Mean: 30.6 CPM, CI95: 30.4 - 30.9

 

 

To get a rough approximation of the radiation contribution of the fossil I subtracted the background radiation:

 

Differential CPM

02 cm: Mean: 51.3 CPM

04 cm: Mean: 27.5 CPM

08 cm: Mean: 11.1 CPM

16 cm: Mean:  3.6 CPM

32 cm: Mean:  0.9 CPM

 

 

The Inverse-square law tells us that if the radiation sensed by the tube should be proportional to the inverse of the squared distance:

 

 

So duplicating the distance reduces the radiation flux to 1 / 4. I used the previous differential data to calculate the radiation reduction:

 

CPM reduction

02 cm -> 04 cm: 1 / 1.9

04 cm -> 08 cm: 1 / 2.5

08 cm -> 16 cm: 1 / 3.1

16 cm -> 32 cm: 1 / 3.9

 

 

As it can be seen only from 16 to 32 cm the reduction was close to the expected 1 / 4. This is because the law applies only "point sources", and the farther the distance the more the source approximates to a point. Instead of measuring the radiation for a specific distance, it is also possible to do the opposite exercise: measure the distance by measuring the radiation flux. This would allow us to use multiple Geiger tubes to compute the position in space of a a radioactive object through trilateration.

 

 

Radiation blocking

 

Just for fun I tested 2 barriers in-between the radiation source and the tube: a 1.85 mm wide plastic ruler and a 0.5 wide metallic box:

 

 

 

Absolute CPM

Background: 29.7 CPM

Unblocked:  57.2 CPM

Ruler:      48.1 CPM

Box:        43.8 CPM

 

 

I subtracted the background and also computed how much radiation flew through the barrier to the tube:

 

Differential CPM

Unblocked: 27.4 CPM

Ruler:     18.4 CPM (67.1%)

Box:       14.1 CPM (51.4%)

 

 

As it can be seen the metal box blocks more than 3 times the amount of radiation per width than the plastic ruler. These experiments could have been much more interesting, for instance I would have liked to test different metals, but sadly I didn't have much around to perform more interesting experiments.

 

 

Final words

 

I built the Geiger counter long ago but never performed any measurements until now. Even though the results that I got were more or less expected, its always rewarding to see how the theory works in the practice. Most of these experiments were very rough and lots of assumptions had to be made, for instance radiation emitted by the barriers was assumed to be negligible, as any barrier emission would have contaminated the results.

 

Besides using radioactivity to compute the position of a radioactive object in space, another interesting, but not very practical use for a radiation source and Geiger counter is to generate random numbers. One way to generate them is to measure 2 consecutive intervals and if the first one is larger than the second one, generate a bit with a 0, while if the second interval is larger the first one, generate a bit with a 1. In this way 1 bit is generated every 2 counts, so at the maximum rate that I got of 237.5 CPM, I could generate 1.98 random bits per second (ie: 16 s would be required to generate a random 32-bit integer).

Anonymous

Top Comments

  • Jan Cumps
    Jan Cumps over 1 year ago in reply to jw0752 +6

    Bright orange stoneware (plates, cups) made first part of the 20th century (say up to the late 1930s - mid 40s) may radiate too.

  • jw0752
    jw0752 over 1 year ago in reply to neuromodulator +6

    Here are a couple pictures of my unit:

     

     

     

    It seems I bought it in 1973 from a company called Edmund Scientific. I guess I paid a couple hundred dollars at the time. I did not have the electronic skills to…

  • jw0752
    jw0752 over 1 year ago +5

    This is a great experiment and I enjoyed reading about it. I was wondering if you can give a little more background on how you measured the 68k events over a 38 hour period. When I was younger they were…

  • neuromodulator
    neuromodulator over 1 year ago in reply to Jan Cumps

    Very interesting Jan, Wikipedia has some interesting information on the use of pralidoxime+atropine: https://en.wikipedia.org/wiki/Pralidoxime . Apparently most nerve are organophosphates, and could be treated with that antidote

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  • Jan Cumps
    Jan Cumps over 1 year ago

    When I was in the army 2nd half of the 80s and moved to West-Germany, we all had an aluminum tube with a clip in our jacket pocket. To be worn all time when in duty.

    If you unscrewed it, there was a valve in there, to collect the radiation level over time. There was nothing else in there except protection to avoid the tube from breaking.

    They were not supposed to be used for checking individual soldier's levels. Would be collected for the whole battery together without info on who used a particular pen.

     

    I tried to google for an image but didn't get a result that looked like the thing yet.

     

    edit: this is the closest I could find:

     

    Edit edit: also had something like this in the same pocket, but also in a aluminum pen-style tube:

    That's for when you become victim of nerve agent.

    Because in that case you have no muscle control, you have to hope that someone sees you, finds the pen in your pocket and shoots the antidote in your upper leg through your pants.

    Then they have to hang the pen on the outside of your pocket, to indicate you've been antidoted. Because two of these injections aren't good-for-ya.

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  • jc2048
    jc2048 over 1 year ago

    That's an interesting looking G-M tube. I've got one that I bought years ago (1970s - they were sold as

    'surplus' at the time, so I don't suppose it cost me very much), but I never did anything with it.

     

     

    This one was intended for use with a piece of British civil defence equipment. It has a rubber boot around

    it to give some protection and the base is in the form of a plug with two terminals. That allowed the tubes

    to be changed easily [from looking online, it seems that there was also a specialised one that had a tray

    for testing drinking water samples].

     

    Helpfully, it has the operating voltage printed on it. Perhaps I should give it a try and see if it works.

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  • neuromodulator
    neuromodulator over 1 year ago in reply to jw0752

    I would have thought in the middle of the cold war these things would have sold at a very low cost almost at any shop. Your scintillator has the same form-factor than many others that I've seen on eBay, except that for some reason they usually are yellow.

    I posted an image that shows how everything was configured, not sure if it displayed on your end (some time ago I had some trouble with some images that were only visible to me).

     

    The input voltage is 6 V DC, so that I could use 4 AA batts, but here I just connected it to a small 6 V power supply. I then boost-converted the voltage to 400 V, this was not done in the most efficient way (I used some scrap I had laying around). The 400 V is what the Geiger tube (mine is not a scintillator) needs to see, and while no event gets detected, it stays non-conductive (I was not able to measure resistance with my SMU, so it might be in the Teraohm range), when an event gets detected it turns conductive (haven't measured how conductive) . A voltage divider in series with the tube generates an output of ∼3 V when an event occurs. The divider is set to have high impedance so that it reduces the current and the draining of the capacitor that is keeping the 400 V output to the tube. The pulses last around 0.5 ms and are samples with the ADC of an Arduino, the Arduino is connected to a Raspberry Pi that runs a Python program to read the serial port and store the data. The only purpose of the Raspberry Pi was to save electricity, as leaving the computer on for so many days on would have cost me quite a bit (All the experiments took me several days of continuous recording).

     

    I will upload the Arduino and Python code to make it available...

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  • jw0752
    jw0752 over 1 year ago in reply to neuromodulator

    Here are a couple pictures of my unit:

     

     

     

    It seems I bought it in 1973 from a company called Edmund Scientific. I guess I paid a couple hundred dollars at the time. I did not have the electronic skills to build one and of course we did not even have cell phones let alone an internet where I could get any instructions. I have played with it off and on over the years but I was foolish to spend that much for it back then and my opinion of the purchase hasn't changed over the years. I probably wouldn't even be here now if the wife had discovered what I paid for it.

     

    My question was on how you configured your test equipment to turn it into a scintillation counter whereby you were able to log the number of events over the 38 hour period.

     

    John

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